Deformation and mixing of coexisting shapes in neutron-deficient polonium isotopes
Phys. Rev. C
Coulomb-excitation experiments are performed with postaccelerated beams of neutron-deficient
196,198,200,202
Po
isotopes at the REX-ISOLDE facility. A set of matrix elements, coupling the low-lying states in these isotopes, is extracted. In the two heaviest isotopes,
200,202
Po
, the transitional and diagonal matrix elements of the 2+
1 state are determined. In
196,198
Po
multistep Coulomb excitation is observed, populating the 4+
1,0+
2, and 2+
2 states. The experimental results are compared to the results from the measurement of mean-square charge radii in polonium isotopes, confirming the onset of deformation from
196
Po
onwards. Three model descriptions are used to compare to the data. Calculations with the beyond-mean-field model, the interacting boson model, and the general Bohr Hamiltonian model show partial agreement with the experimental data. Finally, calculations with a phenomenological two-level mixing model hint at the mixing of a spherical structure with a weakly deformed rotational structure.